Synthetische Zugange Zum A, B, C-Ringsystem Des Naturstoffes Beticolin 0 Durch Regioselektive Naphthochinon-Diels-Alder-Reaktionen
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Synthetische Zugange Zum A, B, C-Ringsystem Des Naturstoffes Beticolin 0 Durch Regioselektive Naphthochinon-Diels-Alder-Reaktionen

Synthetische Zugange Zum A, B, C-Ringsystem Des Naturstoffes Beticolin 0 Durch Regioselektive Naphthochinon-Diels-Alder-Reaktionen


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About the Book

Die Beticoline sind Mykotoxine, die von dem Pilz Cercospora beticola produziert werden. Diese Pilzgattung wird verantwortlich gemacht fur die Blattfleckenkrankheit von Zuckerruben (Cercosporiose), die eine grosse okonomische Bedeutung fur die Agrarindustrie hat. Einige Beticoline zeigen dazu potente Antitumor-Eigenschaften und andere interessante biologische Effekte. Bis heute konnten 20 Beticoline isoliert werden, dazu wurden weitere Naturstoffe beschrieben, welche eine hohe strukturelle Ahnlichkeit aufweisen. Die Beticoline teilen ein polyzyklisches Grundgerust: Ein zentrales Bicyclo[3.2.2]nonan-Ringsystem wird von einer monochlorierten Xanthon- und einer Tetrahydroanthrachinon-Untereinheit flankiert. In der vorliegenden Arbeit konnte der A, B, C-Trizyklus von Beticolin 0, welcher der Tetrahydroanthrachinon-Untereinheit entspricht, durch drei verschiedene Methoden synthetisiert werden. Mit der Synthese dieser Untereinheit wurde auch das quartare Zentrum des Naturstoffs konstruiert. Im Rahmen dieser Dissertation wurden wichtige Grundlagen hinsichtlich der Totalsynthese der Beticoline gelegt. Ebenso wurden einige der hergerstellten Stoffe in Zytotoxizitatsassays untersucht und dabei ausserst potente Substanzen ermittelt.


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Product Details
  • ISBN-13: 9783832536671
  • Publisher: Logos Verlag Berlin
  • Binding: Paperback
  • Language: German
  • Returnable: N
  • Spine Width: 0 mm
  • Width: 145 mm
  • ISBN-10: 3832536671
  • Publisher Date: 15 Apr 2014
  • Height: 210 mm
  • No of Pages: 210
  • Series Title: Beitrage Zur Organischen Synthese
  • Weight: 750 gr


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Synthetische Zugange Zum A, B, C-Ringsystem Des Naturstoffes Beticolin 0 Durch Regioselektive Naphthochinon-Diels-Alder-Reaktionen
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